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Local negative permittivity and topological phase transition in polar skyrmions

Abstract: Topological solitons such as magnetic skyrmions have drawn attention as stable quasi-particle-like objects. The recent Discovery of polar vortices and skyrmions in ferroelectric oxide superlattices has opened up new vistas to explore topology, emergent phenomena and approaches for manipulating such features with electric fields. Using macroscopic dielectric measurements, coupled with direct scanning convergent beam electron diffraction imaging on the atomic scale, theoretical phase-field simulations and second-principles calculations, we demonstrate that polar skyrmions in (PbTiO3)n/(SrTiO3)n superlattices are distinguished by a sheath of negative permittivity at the periphery of each skyrmion. This enhances the effective dielectric permittivity compared with the individual SrTiO3 and PbTiO3 layers. Moreover, the response of these topologically protected structures to electric field and temperature shows a reversible phase transition from the skyrmion state to a trivial uniform ferroelectric state, accompanied by large tunability of the dielectric permittivity. Pulsed switching measurements show a time-dependent evolution and recovery of the skyrmion state (and macroscopic dielectric response). The interrelationship between topological and dielectric properties presents an opportunity to simultaneously manipulate both by a single, and easily controlled, stimulus, the applied electric field.

 Autoría: Das S., Hong Z., Stoica V.A., Gonçalves M.A.P., Shao Y.T., Parsonnet E., Marksz E.J., Saremi S., McCarter M.R., Reynoso A., Long C.J., Hagerstrom A.M., Meyers D., Ravi V., Prasad B., Zhou H., Zhang Z., Wen H., Gómez-Ortiz F., García-Fernández P., Bokor J., Íñiguez J., Freeland J.W., Orloff N.D., Junquera J., Chen L.Q., Salahuddin S., Muller D.A., Martin L.W., Ramesh R.,

 Fuente: Nature Materials, 2021, 20(2), 194-201 - (CORRIGENDUM), 2021, 20(6), 905

Editorial: Nature Publishing Group

 Fecha de publicación: 01/02/2021

Nº de páginas: 21

Tipo de publicación: Artículo de Revista

 DOI: 10.1038/s41563-020-00818-y

ISSN: 1476-1122,1476-4660

 Proyecto español: FIS2015-64886-C5-2-P

Url de la publicación: https://doi.org/10.1038/s41563-020-00818-y

Autoría

DAS, S.

HONG, Z.

STOICA, V. A.

GONÇALVES, M.A.P.

SHAO, Y. T.

PARSONNET, E.

MARKSZ, E. J.

SAREMI, S.

MCCARTER, M. R.

REYNOSO, A.

LONG, C. J.

HAGERSTROM, A. M.

MEYERS, D.

V. RAVI

PRASAD, B.

ZHOU, H.

Z. ZHANG

FERNANDO GOMEZ ORTIZ