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Coupling between tilts and charge carriers at polar-nonpolar perovskite interfaces

Abstract: The phenomenological theory for the polar instability giving rise to a two-dimensional electron gas at perovskite interfaces is hereby extended to include the coupling to perovskite tilts. A Landau theory for homogeneous tilts is first explored, setting the scene for the further, more realistic Landau-Ginzburg theory describing varying tilt amplitudes across a thin film. The theory is also generalized to account for the response to an applied electric field normal to the interface, which allows a finer control on phase transitions. The conventionally described physics of a single metal-insulator transition is substantially enriched by the coupling, the model describing various scenarios with one or two transitions, possibly continuous or discontinuous. First-principles calculations permit the estimation of the parameters defining the model, which have been calculated for the interface between lanthanum aluminate and strontium titanate.

Other publications of the same journal or congress with authors from the University of Cantabria

 Fuente: Physical Review B, 2022, 106(9), 094106

Publisher: American Physical Society

 Publication date: 01/09/2022

No. of pages: 16

Publication type: Article

 DOI: 10.1103/PhysRevB.106.094106

ISSN: 1098-0121,1550-235X,2469-9950,2469-9969

 Spanish project: CEX2020-001038-M

Publication Url: https://doi.org/10.1103/PhysRevB.106.094106

Authorship

BENNETT, DANIEL

ARTACHO, EMILIO

BRISTOWE, NICHOLAS C.